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Novel opportunities for sub-meV inelastic X-ray scattering at high-repetition rate self-seeded X-ray free-electron lasers

机译:亚微米非弹性X射线散射的新机会   高重复率自种X射线自由电子激光器

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摘要

Inelastic X-ray scattering (IXS) is an important tool for studies ofequilibrium dynamics in condensed matter. A new spectrometer recently proposedfor ultra-high-resolution IXS (UHRIX) has achieved 0.6~meV and 0.25~nm$^{-1}$spectral and momentum transfer resolutions, respectively. However, furtherimprovements down to 0.1~meV and 0.02~nm$^{-1}$ are required to close the gapin energy-momentum space between high and low frequency probes. We show thatthis goal can be achieved by further optimizing the X-ray optics and byincreasing the spectral flux of the incident X-ray pulses. UHRIX performs bestat energies from 5 to 10 keV, where a combination of self-seeding and undulatortapering at the SASE-2 beamline of the European XFEL promises up to ahundred-fold increase in average spectral flux compared with nominal SASEpulses at saturation, or three orders of magnitude more than possible withstorage-ring based radiation sources. Wave-optics propagation shows that about$7\times 10^{12}$~ph/s in a $90$-$\mu$eV bandwidth can be achieved on thesample. This will provide unique new possibilities for dynamics studies by IXS.
机译:非弹性X射线散射(IXS)是研究凝聚态平衡动力学的重要工具。最近针对超高分辨率IXS(UHRIX)提出的新光谱仪已实现了0.6〜meV和0.25〜nm $ ^ {-1} $的光谱和动量传递分辨率。然而,需要进一步降低至0.1〜meV和0.02〜nm $ ^ {-1} $的水平,以弥合高频和低频探头之间的能量动量空间。我们表明,可以通过进一步优化X射线光学系统并增加入射X射线脉冲的光谱通量来实现此目标。 UHRIX执行的bestat能量为5到10 keV,其中欧洲XFEL的SASE-2光束线上的自播和起伏锥形相结合,可使平均光谱通量与饱和时的标称SASE脉冲相比增加多达数百倍,或三个数量级远远超过基于存储环的辐射源。波光学传播表明,在90美元-美元/亩-eV带宽中,可以实现大约7美元乘以10 ^ {12} $ ph / s。这将为IXS的动力学研究提供独特的新可能性。

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